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Final published version
The ultrafast dynamics of short-pulse-laser-excited fused silica is investigated by measuring polarization-resolved reflectances of a wavelength-tunable probe pulse following a near-infrared pump pulse. These data, which should, in principle, allow the determination of both real and imaginary parts of the time-dependent electric permittivity, turn out to become incompatible with an isotropic optical response after ∼200 fs. This is reconciled with a uniaxial permittivity tensor, which predicts greatly enhanced absorption of p-polarized light, suggesting that an absorption channel is missing in the standard optical models for strongly excited dielectrics. The timescale for the excitation-induced variations in the optical properties exhibits a wavelength dependence that can be explained qualitatively by Pauli blocking in the electronic band structure.
Original language | English |
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Article number | 043010 |
Journal | Physical Review Research |
Volume | 2 |
Issue | 4 |
ISSN | 2643-1564 |
DOIs | |
Publication status | Published - Oct 2020 |
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ID: 197835780