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We present theoretical results for intensity-dependent above-threshold ionization (ATI) spectra from oriented OCS molecules probed by intense femtosecond laser pulses with wavelengths of 800 and 400 nm. The calculations were performed using the time-dependent Schrödinger equation within the single-active-electron approximation and including multielectron polarization effects. The results capture some of the experimental findings (Yu et al 2017 J. Phys. B: At. Mol. Opt. Phys. 50 235602), in particular when considering the sensitivity of the ATI spectra on the molecular orientation. We identify characteristic features in the ATI spectra which correspond to resonant multiphoton ionization via highly-excited Rydberg states are captured by the theory.
Original language | English |
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Article number | 105401 |
Journal | Journal of Physics B: Atomic, Molecular and Optical Physics |
Volume | 56 |
Issue | 10 |
ISSN | 0953-4075 |
DOIs | |
Publication status | Published - Apr 2023 |
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