State of knowledge on current exposure, fate and potential health effects of contaminants in polar bears from the circumpolar Arctic

Heli Routti*, Todd C. Atwood, Thea Bechshoft, Andrei Boltunov, Tomasz M. Ciesielski, Jean Pierre Desforges, Rune Dietz, Geir W. Gabrielsen, Bjørn M. Jenssen, Robert J. Letcher, Melissa A. McKinney, Adam D. Morris, Frank F. Rigét, Christian Sonne, Bjarne Styrishave, Sabrina Tartu

*Corresponding author for this work

Research output: Contribution to journal/Conference contribution in journal/Contribution to newspaperReviewResearchpeer-review

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Abstract

The polar bear (Ursus maritimus) is among the Arctic species exposed to the highest concentrations of long-range transported bioaccumulative contaminants, such as halogenated organic compounds and mercury. Contaminant exposure is considered to be one of the largest threats to polar bears after the loss of their Arctic sea ice habitat due to climate change. The aim of this review is to provide a comprehensive summary of current exposure, fate, and potential health effects of contaminants in polar bears from the circumpolar Arctic required by the Circumpolar Action Plan for polar bear conservation. Overall results suggest that legacy persistent organic pollutants (POPs) including polychlorinated biphenyls, chlordanes and perfluorooctane sulfonic acid (PFOS), followed by other perfluoroalkyl compounds (e.g. carboxylic acids, PFCAs) and brominated flame retardants, are still the main compounds in polar bears. Concentrations of several legacy POPs that have been banned for decades in most parts of the world have generally declined in polar bears. Current spatial trends of contaminants vary widely between compounds and recent studies suggest increased concentrations of both POPs and PFCAs in certain sub populations. Correlative held studies, supported by in vitro studies, suggest that contaminant exposure disrupts circulating levels of thyroid hormones and lipid metabolism, and alters neurochemistry in polar bears. Additionally, field and in vitro studies and risk assessments indicate the potential for adverse impacts to polar bear immune functions from exposure to certain contaminants. (C) 2019 Elsevier B.V. All rights reserved.

Original languageEnglish
JournalScience of the Total Environment
Volume664
Pages (from-to)1063-1083
Number of pages21
ISSN0048-9697
DOIs
Publication statusPublished - 10 May 2019

Keywords

  • Emerging compounds
  • Mercury
  • Persistent organic pollutants
  • PFAS
  • Pollutant
  • Ursus maritimus
  • ENDOCRINE-DISRUPTING CHEMICALS
  • POLYFLUOROALKYL SUBSTANCES PFASS
  • PEAS
  • 3 DECADES 1983-2010
  • BONE-MINERAL DENSITY
  • SOUTHERN BEAUFORT SEA
  • PERSISTENT ORGANIC POLLUTANTS
  • GLOBAL EMISSION INVENTORIES
  • POLYBROMINATED DIPHENYL ETHERS
  • CHLORINATED-HYDROCARBON CONTAMINANTS
  • LONG-RANGE TRANSPORT

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