Sintering in seconds, elucidated by millisecond in situ diffraction

Priyank Shyam; Frederik H. Gjørup; Mathias I. Mørch; Amalie P. Laursen; Anna Z. Eikeland; Innokenty Kantor; Mads R.V. Jørgensen; Mogens Christensen

doi:10.1016/j.apmt.2023.101960

Sintering in seconds, elucidated by millisecond in situ diffraction

Priyank Shyam, Frederik H. Gjørup, Mathias I. Mørch, Amalie P. Laursen, Anna Z. Eikeland, Innokenty Kantor, Mads R.V. Jørgensen, Mogens Christensen^*

^*Corresponding author for this work

Research output: Contribution to journal/Conference contribution in journal/Contribution to newspaper › Journal article › Research › peer-review

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Abstract

Materials, when sintered at high temperatures, undergo structural changes on multiple, hierarchical length scales but getting realtime information on these changes is difficult. To address this challenge, we developed a custom-built sample environment that allows us to investigate the structural evolution of materials during sintering using high-energy two-dimensional synchrotron X-ray diffraction (2D-XRD). Changes in the structure of SrFe₁₂O₁₉ ceramic magnet at multiple length scales were tracked in situ and modelled with millisecond time-resolution. In addition, we also demonstrated the ability to perform quantitative texture analysis from individual 2D-XRD images with a time resolution of 4 ms each. Owing to the high brightness X-ray source and advanced X-ray detectors, the evolution of crystallographic texture could be followed during sintering. This in situ approach can aid understanding of the synthesis–structure–property relationships in sintered materials, enabling the development of improved functional materials.

Original language	English
Article number	101960
Journal	Applied Materials Today
Volume	35
Number of pages	9
DOIs	https://doi.org/10.1016/j.apmt.2023.101960
Publication status	Published - Dec 2023

Keywords

Functional materials
In situ diffraction
Sintering
Texture
Time-resolved

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1-s2.0-S2352940723002305-mainFinal published version, 4.19 MBLicence: CC BY

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title = "Sintering in seconds, elucidated by millisecond in situ diffraction",

abstract = "Materials, when sintered at high temperatures, undergo structural changes on multiple, hierarchical length scales but getting realtime information on these changes is difficult. To address this challenge, we developed a custom-built sample environment that allows us to investigate the structural evolution of materials during sintering using high-energy two-dimensional synchrotron X-ray diffraction (2D-XRD). Changes in the structure of SrFe12O19 ceramic magnet at multiple length scales were tracked in situ and modelled with millisecond time-resolution. In addition, we also demonstrated the ability to perform quantitative texture analysis from individual 2D-XRD images with a time resolution of 4 ms each. Owing to the high brightness X-ray source and advanced X-ray detectors, the evolution of crystallographic texture could be followed during sintering. This in situ approach can aid understanding of the synthesis–structure–property relationships in sintered materials, enabling the development of improved functional materials.",

keywords = "Functional materials, In situ diffraction, Sintering, Texture, Time-resolved",

author = "Priyank Shyam and Gj{\o}rup, {Frederik H.} and M{\o}rch, {Mathias I.} and Laursen, {Amalie P.} and Eikeland, {Anna Z.} and Innokenty Kantor and J{\o}rgensen, {Mads R.V.} and Mogens Christensen",

note = "Publisher Copyright: {\textcopyright} 2023 The Author(s)",

year = "2023",

month = dec,

doi = "10.1016/j.apmt.2023.101960",

language = "English",

volume = "35",

journal = "Applied Materials Today",

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AU - Shyam, Priyank

AU - Gjørup, Frederik H.

AU - Mørch, Mathias I.

AU - Laursen, Amalie P.

AU - Eikeland, Anna Z.

AU - Kantor, Innokenty

AU - Jørgensen, Mads R.V.

AU - Christensen, Mogens

PY - 2023/12

Y1 - 2023/12

N2 - Materials, when sintered at high temperatures, undergo structural changes on multiple, hierarchical length scales but getting realtime information on these changes is difficult. To address this challenge, we developed a custom-built sample environment that allows us to investigate the structural evolution of materials during sintering using high-energy two-dimensional synchrotron X-ray diffraction (2D-XRD). Changes in the structure of SrFe12O19 ceramic magnet at multiple length scales were tracked in situ and modelled with millisecond time-resolution. In addition, we also demonstrated the ability to perform quantitative texture analysis from individual 2D-XRD images with a time resolution of 4 ms each. Owing to the high brightness X-ray source and advanced X-ray detectors, the evolution of crystallographic texture could be followed during sintering. This in situ approach can aid understanding of the synthesis–structure–property relationships in sintered materials, enabling the development of improved functional materials.

AB - Materials, when sintered at high temperatures, undergo structural changes on multiple, hierarchical length scales but getting realtime information on these changes is difficult. To address this challenge, we developed a custom-built sample environment that allows us to investigate the structural evolution of materials during sintering using high-energy two-dimensional synchrotron X-ray diffraction (2D-XRD). Changes in the structure of SrFe12O19 ceramic magnet at multiple length scales were tracked in situ and modelled with millisecond time-resolution. In addition, we also demonstrated the ability to perform quantitative texture analysis from individual 2D-XRD images with a time resolution of 4 ms each. Owing to the high brightness X-ray source and advanced X-ray detectors, the evolution of crystallographic texture could be followed during sintering. This in situ approach can aid understanding of the synthesis–structure–property relationships in sintered materials, enabling the development of improved functional materials.

KW - Functional materials

KW - In situ diffraction

KW - Sintering

KW - Texture

KW - Time-resolved

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U2 - 10.1016/j.apmt.2023.101960

DO - 10.1016/j.apmt.2023.101960

M3 - Journal article

AN - SCOPUS:85174723529

SN - 2352-9415

VL - 35

JO - Applied Materials Today

JF - Applied Materials Today

M1 - 101960

ER -

Sintering in seconds, elucidated by millisecond in situ diffraction

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Keywords

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