Multielectron effects in strong-field ionization of the oriented OCS molecule

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We present theoretical calculations of orientation-dependent total ionization yields from the highest occupied molecular orbitals of the oriented OCS molecule by solving the time-dependent Schrödinger equation in three dimensions. The calculations were performed within the single-active-electron approximation including multielectron polarization. The multielectron polarization term was represented by an induced dipole term which contains the polarizability of the OCS+ cation parallel to the laser polarization. Upon accounting for multielectron polarization, the calculated total ionization yields and their orientation dependence are in good agreement with experimental data.

Original languageEnglish
Article number063111
JournalPhysical Review A
Volume102
Issue6
ISSN2469-9926
DOIs
Publication statusPublished - Dec 2020

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