Research output: Contribution to journal/Conference contribution in journal/Contribution to newspaper › Journal article › Research › peer-review
Centimeter-sized 2D alpha-MoO3 single crystal : growth, Raman anisotropy, and optoelectronic properties. / Zheng, Binjie; Wang, Zegao; Chen, Yuanfu; Zhang, Wanli; Li, Xuesong.
In: 2D materials, Vol. 5, No. 4, 045011, 25.07.2018.Research output: Contribution to journal/Conference contribution in journal/Contribution to newspaper › Journal article › Research › peer-review
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TY - JOUR
T1 - Centimeter-sized 2D alpha-MoO3 single crystal
T2 - growth, Raman anisotropy, and optoelectronic properties
AU - Zheng, Binjie
AU - Wang, Zegao
AU - Chen, Yuanfu
AU - Zhang, Wanli
AU - Li, Xuesong
PY - 2018/7/25
Y1 - 2018/7/25
N2 - Centimeter-sized 2D layered alpha-MoO3 single crystal has been grown by a facile physical vapor deposition method. The lateral size of alpha-MoO3 single crystals can be tunable from micrometer to centimeter by controlling the inner diameter of the quartz tube reaction chamber. The as-grown alpha-MoO3 exhibits strong in-plane Raman anisotropy, where A(g) Raman modes give the direction of crystallographic orientation, which can be used to rapidly and precisely identify the crystallinity of large-area alpha-MoO3 through selected-area angel-resolved polarized Raman spectroscopy. Moreover, the photodetectors based on annealed alpha-MoO3 single crystals exhibit excellent optoelectronic performance with a photoresponsivity of 65.6 A W-1 and a fast photoresponse time of 2 s.
AB - Centimeter-sized 2D layered alpha-MoO3 single crystal has been grown by a facile physical vapor deposition method. The lateral size of alpha-MoO3 single crystals can be tunable from micrometer to centimeter by controlling the inner diameter of the quartz tube reaction chamber. The as-grown alpha-MoO3 exhibits strong in-plane Raman anisotropy, where A(g) Raman modes give the direction of crystallographic orientation, which can be used to rapidly and precisely identify the crystallinity of large-area alpha-MoO3 through selected-area angel-resolved polarized Raman spectroscopy. Moreover, the photodetectors based on annealed alpha-MoO3 single crystals exhibit excellent optoelectronic performance with a photoresponsivity of 65.6 A W-1 and a fast photoresponse time of 2 s.
KW - two-dimensional semiconductor
KW - physical vapor deposition
KW - molybdenum trioxide
KW - Raman anisotropy
KW - photoresponse
KW - BLACK PHOSPHORUS
KW - MOLYBDENUM OXIDE
KW - NANOSHEETS
KW - SPECTROSCOPY
KW - DEPENDENCE
KW - SCATTERING
KW - MECHANISM
KW - GRAPHENE
KW - MOS2
U2 - 10.1088/2053-1583/aad2ba
DO - 10.1088/2053-1583/aad2ba
M3 - Journal article
VL - 5
JO - 2D materials
JF - 2D materials
SN - 2053-1583
IS - 4
M1 - 045011
ER -