Research output: Contribution to journal/Conference contribution in journal/Contribution to newspaper › Journal article › Research › peer-review
2D SnSe/Si heterojunction for self-driven broadband photodetectors. / Hao, Lanzhong; Wang, Zegao; Xu, Hanyang; Yan, Keyou; Dong, Shichang; Liu, Hui; Du, Yongjun; Wu, Yupeng; Liu, Yunjie; Dong, Mingdong.
In: 2D materials, Vol. 6, No. 3, 034004, 05.2019.Research output: Contribution to journal/Conference contribution in journal/Contribution to newspaper › Journal article › Research › peer-review
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TY - JOUR
T1 - 2D SnSe/Si heterojunction for self-driven broadband photodetectors
AU - Hao, Lanzhong
AU - Wang, Zegao
AU - Xu, Hanyang
AU - Yan, Keyou
AU - Dong, Shichang
AU - Liu, Hui
AU - Du, Yongjun
AU - Wu, Yupeng
AU - Liu, Yunjie
AU - Dong, Mingdong
PY - 2019/5
Y1 - 2019/5
N2 - Van der Waals heterojunctions based on atomically thin 2D materials have opened up new realms in modern semiconductor industry. However, it is still challenging to fabricate large-area ultrathin 2D films. Herein, we successfully fabricate wafer-size 2D SnSe films on Si substrate by magnetron sputtering technique, enabling the formation of SnSe/Si van der Waals (vdWs) heterojunction device. The high-resolution transmission electron microscopy is employed to character the structure of SnSe film and SnSe/Si heterojunction with ideal orthorhombic structure and atomically abrupt interface, respectively. The energy diagram of SnSe/Si heterojunction is constructed, exhibiting similar barrier heights for electron and hole carrier. The SnSe/Si heterojunction shows obvious diode behavior with rectification ratio of ∼1.6 ×10 4 , forward current of ∼194.5 mA cm -2 at ±1.0 V. Furthermore, owing to the high crystalline orientation, specific energy-band alignment, as well as the strong built-in electrical field, the SnSe/Si heterojunction illustrates a broadband photodetecting properties with the wavelength ranging from ultraviolet to near-infrared light, showing a high detectivity of 4.4 ×10 12 cmHz 1/2 W -1 , a high responsivity of 566.4 mA mW -1 and an ultrafast response/recovery time of ∼1.6/47.7 s under zero external bias. This work provides a new strategy for fabrication of low cost 2D optoelectronic devices with high-performance.
AB - Van der Waals heterojunctions based on atomically thin 2D materials have opened up new realms in modern semiconductor industry. However, it is still challenging to fabricate large-area ultrathin 2D films. Herein, we successfully fabricate wafer-size 2D SnSe films on Si substrate by magnetron sputtering technique, enabling the formation of SnSe/Si van der Waals (vdWs) heterojunction device. The high-resolution transmission electron microscopy is employed to character the structure of SnSe film and SnSe/Si heterojunction with ideal orthorhombic structure and atomically abrupt interface, respectively. The energy diagram of SnSe/Si heterojunction is constructed, exhibiting similar barrier heights for electron and hole carrier. The SnSe/Si heterojunction shows obvious diode behavior with rectification ratio of ∼1.6 ×10 4 , forward current of ∼194.5 mA cm -2 at ±1.0 V. Furthermore, owing to the high crystalline orientation, specific energy-band alignment, as well as the strong built-in electrical field, the SnSe/Si heterojunction illustrates a broadband photodetecting properties with the wavelength ranging from ultraviolet to near-infrared light, showing a high detectivity of 4.4 ×10 12 cmHz 1/2 W -1 , a high responsivity of 566.4 mA mW -1 and an ultrafast response/recovery time of ∼1.6/47.7 s under zero external bias. This work provides a new strategy for fabrication of low cost 2D optoelectronic devices with high-performance.
KW - broadband
KW - heterojunction
KW - photodetector
KW - self-driven
KW - tin monoselenide
UR - http://www.scopus.com/inward/record.url?scp=85065641897&partnerID=8YFLogxK
U2 - 10.1088/2053-1583/ab15f7
DO - 10.1088/2053-1583/ab15f7
M3 - Journal article
AN - SCOPUS:85065641897
VL - 6
JO - 2D materials
JF - 2D materials
SN - 2053-1583
IS - 3
M1 - 034004
ER -