Exploring the potential of MXene nanohybrids as high-performance anode materials for lithium-ion batteries

Narendra Bandaru; Ch Venkata Reddy; Kalyani Vallabhudasu; Mule Vijayalakshmi; Kakarla Raghava Reddy; Bai Cheolho; Jaesool Shim; Tejraj M. Aminabhavi

doi:10.1016/j.cej.2024.157317

Exploring the potential of MXene nanohybrids as high-performance anode materials for lithium-ion batteries

Narendra Bandaru, Ch Venkata Reddy^*, Kalyani Vallabhudasu, Mule Vijayalakshmi, Kakarla Raghava Reddy^*, Bai Cheolho, Jaesool Shim, Tejraj M. Aminabhavi

^*Corresponding author af dette arbejde

Institut for Elektro- og Computerteknologi - Electronics and Photonics

Publikation: Bidrag til tidsskrift/Konferencebidrag i tidsskrift /Bidrag til avis › Tidsskriftartikel › Forskning › peer review

2 Citationer (Scopus)

Abstract

Lithium-ion batteries (LIBs) are an integral part of modern life, powering diverse applications from transportable devices to electric vehicles. Efficacy of LIBs depends on the performance of their components with anode material playing the pivotal role. Traditional graphite anodes have limitations in capacity and rate capability. This review comprehensively discusses utilization of MXene-based composites as anode materials in LIBs. MXene composites exhibit versatile lithium storage mechanisms, involving intercalation and/or conversion reactions. Pure MXenes offer advantages of high capacity and cycling stability having challenges due to limited conductivity and mechanical fragility, restricting their practical utility, thereby affecting their performance in solid-state polymer electrolytes (SPEs). MXene composites overcome unsystematic dispersal and accumulation issues of pure MXene. MXenes in composite form could increase LIBs performance by overcoming limitations of pure MXenes, enabling breakthroughs in energy storage. The review covers different MXene composites viz., MXene/graphene, MXene/silicon, MXene/tin, MXene/carbon, MXene/metal oxide, and MXene/conducting polymer providing a holistic overview. Their performance, cycling stability, and rate capability are discussed to cover challenges and future prospects.

Originalsprog	Engelsk
Artikelnummer	157317
Tidsskrift	Chemical Engineering Journal
Vol/bind	500
ISSN	1385-8947
DOI	https://doi.org/10.1016/j.cej.2024.157317
Status	Udgivet - nov. 2024

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title = "Exploring the potential of MXene nanohybrids as high-performance anode materials for lithium-ion batteries",

abstract = "Lithium-ion batteries (LIBs) are an integral part of modern life, powering diverse applications from transportable devices to electric vehicles. Efficacy of LIBs depends on the performance of their components with anode material playing the pivotal role. Traditional graphite anodes have limitations in capacity and rate capability. This review comprehensively discusses utilization of MXene-based composites as anode materials in LIBs. MXene composites exhibit versatile lithium storage mechanisms, involving intercalation and/or conversion reactions. Pure MXenes offer advantages of high capacity and cycling stability having challenges due to limited conductivity and mechanical fragility, restricting their practical utility, thereby affecting their performance in solid-state polymer electrolytes (SPEs). MXene composites overcome unsystematic dispersal and accumulation issues of pure MXene. MXenes in composite form could increase LIBs performance by overcoming limitations of pure MXenes, enabling breakthroughs in energy storage. The review covers different MXene composites viz., MXene/graphene, MXene/silicon, MXene/tin, MXene/carbon, MXene/metal oxide, and MXene/conducting polymer providing a holistic overview. Their performance, cycling stability, and rate capability are discussed to cover challenges and future prospects.",

keywords = "Electrochemical properties, Electrode materials, Energy storage, Heterostructured nanohybrids, Lithium-ion batteries, MXenes",

author = "Narendra Bandaru and Reddy, {Ch Venkata} and Kalyani Vallabhudasu and Mule Vijayalakshmi and {Raghava Reddy}, Kakarla and Bai Cheolho and Jaesool Shim and Aminabhavi, {Tejraj M.}",

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AU - Bandaru, Narendra

AU - Reddy, Ch Venkata

AU - Vallabhudasu, Kalyani

AU - Vijayalakshmi, Mule

AU - Raghava Reddy, Kakarla

AU - Cheolho, Bai

AU - Shim, Jaesool

AU - Aminabhavi, Tejraj M.

PY - 2024/11

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N2 - Lithium-ion batteries (LIBs) are an integral part of modern life, powering diverse applications from transportable devices to electric vehicles. Efficacy of LIBs depends on the performance of their components with anode material playing the pivotal role. Traditional graphite anodes have limitations in capacity and rate capability. This review comprehensively discusses utilization of MXene-based composites as anode materials in LIBs. MXene composites exhibit versatile lithium storage mechanisms, involving intercalation and/or conversion reactions. Pure MXenes offer advantages of high capacity and cycling stability having challenges due to limited conductivity and mechanical fragility, restricting their practical utility, thereby affecting their performance in solid-state polymer electrolytes (SPEs). MXene composites overcome unsystematic dispersal and accumulation issues of pure MXene. MXenes in composite form could increase LIBs performance by overcoming limitations of pure MXenes, enabling breakthroughs in energy storage. The review covers different MXene composites viz., MXene/graphene, MXene/silicon, MXene/tin, MXene/carbon, MXene/metal oxide, and MXene/conducting polymer providing a holistic overview. Their performance, cycling stability, and rate capability are discussed to cover challenges and future prospects.

AB - Lithium-ion batteries (LIBs) are an integral part of modern life, powering diverse applications from transportable devices to electric vehicles. Efficacy of LIBs depends on the performance of their components with anode material playing the pivotal role. Traditional graphite anodes have limitations in capacity and rate capability. This review comprehensively discusses utilization of MXene-based composites as anode materials in LIBs. MXene composites exhibit versatile lithium storage mechanisms, involving intercalation and/or conversion reactions. Pure MXenes offer advantages of high capacity and cycling stability having challenges due to limited conductivity and mechanical fragility, restricting their practical utility, thereby affecting their performance in solid-state polymer electrolytes (SPEs). MXene composites overcome unsystematic dispersal and accumulation issues of pure MXene. MXenes in composite form could increase LIBs performance by overcoming limitations of pure MXenes, enabling breakthroughs in energy storage. The review covers different MXene composites viz., MXene/graphene, MXene/silicon, MXene/tin, MXene/carbon, MXene/metal oxide, and MXene/conducting polymer providing a holistic overview. Their performance, cycling stability, and rate capability are discussed to cover challenges and future prospects.

KW - Electrochemical properties

KW - Electrode materials

KW - Energy storage

KW - Heterostructured nanohybrids

KW - Lithium-ion batteries

KW - MXenes

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DO - 10.1016/j.cej.2024.157317

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VL - 500

JO - Chemical Engineering Journal

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Exploring the potential of MXene nanohybrids as high-performance anode materials for lithium-ion batteries

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